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A tropospheric ozone maximum over the Middle East

Qinbin Li; Daniel J. Jacob; Jennifer A. Logan; Isabelle Bey; Robert M. Yantosca; Hongyu Liu; Randall V. Martin; Arlene M. Fiore; Brendan D. Field; Bryan N. Duncan; Valérie Thouret

Title:
A tropospheric ozone maximum over the Middle East
Author(s):
Li, Qinbin
Jacob, Daniel J.
Logan, Jennifer A.
Bey, Isabelle
Yantosca, Robert M.
Liu, Hongyu
Martin, Randall V.
Fiore, Arlene M.
Field, Brendan D.
Duncan, Bryan N.
Thouret, Valérie
Date:
Type:
Articles
Department(s):
Earth and Environmental Sciences
Lamont-Doherty Earth Observatory
Volume:
28
Persistent URL:
Book/Journal Title:
Geophysical Research Letters
Geographic Area:
Middle East
Publisher:
American Geophysical Union
Abstract:
The GEOS-CHEM global 3-D model of tropospheric chemistry predicts a summertime O3 maximum over the Middle East, with mean mixing ratios in the middle and upper troposphere in excess of 80 ppbv. This model feature is consistent with the few observations from commercial aircraft in the region. Its origin in the model reflects a complex interplay of dynamical and chemical factors, and of anthropogenic and natural influences. The anticyclonic circulation in the middle and upper troposphere over the Middle East funnels northern midlatitude pollution transported in the westerly subtropical jet as well as lightning outflow from the Indian monsoon and pollution from eastern Asia transported in an easterly tropical jet. Large-scale subsidence over the region takes place with continued net production of O3 and little mid-level outflow. Transport from the stratosphere does not contribute significantly to the O3 maximum. Sensitivity simulations with anthropogenic or lightning emissions shut off indicate decreases of 20–30% and 10–15% respectively in the tropospheric O3 column over the Middle East. More observations in this region are needed to confirm the presence of the O3 maximum.
Subject(s):
Tropospheric chemistry--Mathematical models
Ozone
Climatic changes--Effect of human beings on
Climatic changes
Atmospheric chemistry
Environmental sciences
Publisher DOI:
https://doi.org/10.1029/2001GL013134
Item views
159
Metadata:
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Suggested Citation:
Qinbin Li, Daniel J. Jacob, Jennifer A. Logan, Isabelle Bey, Robert M. Yantosca, Hongyu Liu, Randall V. Martin, Arlene M. Fiore, Brendan D. Field, Bryan N. Duncan, Valérie Thouret, , A tropospheric ozone maximum over the Middle East, Columbia University Academic Commons, .

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