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A Chinese Imprint in Insoluble Pollutants Recently Deposited in Central Greenland As Indicated by Lead Isotopes

Aloys Jean-Mathias Bory; Wafa Abouchami; Stephen J. G. Galer; Anders Svensson; John N. Christensen; Pierre E. Biscaye

Title:
A Chinese Imprint in Insoluble Pollutants Recently Deposited in Central Greenland As Indicated by Lead Isotopes
Author(s):
Bory, Aloys Jean-Mathias
Abouchami, Wafa
Galer, Stephen J. G.
Svensson, Anders
Christensen, John N.
Biscaye, Pierre E.
Date:
Department(s):
Lamont-Doherty Earth Observatory
Volume:
48
Persistent URL:
Book/Journal Title:
Environmental Science & Technology
Publisher:
American Chemical Society
Abstract:
A unique ∼10 year record of the lead isotopic composition of airborne insoluble particulate matter deposited in central Greenland was extracted from recent snow layers at NorthGRIP (75.1°N, 042.3°W; elevation 2,959 m), spanning the years 1989–2001. Comparison with lead isotopic signatures of both natural and anthropogenic northern hemisphere (NH) aerosol sources shows that human activities must have accounted for most of the insoluble lead deposited on Greenland during the late 1990s, exceeding by far the natural contribution from large Asian mineral dust inputs. Lead isotopes imply predominance with time of European/Canadian sources over U.S.-derived lead, with an admixed signature typical of Chinese anthropogenic lead sources. The relative contribution of the latter shows a marked seasonal increase during spring. Our record also suggests that China’s weight in the overall supply of insoluble pollutants deposited on Greenland was growing over the past decade of the 20th century.
Subject(s):
Environmental sciences
Chemistry
Geochemistry
Publisher DOI:
https://doi.org/10.1021/es4035655
Item views
129
Metadata:
text | xml
Suggested Citation:
Aloys Jean-Mathias Bory, Wafa Abouchami, Stephen J. G. Galer, Anders Svensson, John N. Christensen, Pierre E. Biscaye, , A Chinese Imprint in Insoluble Pollutants Recently Deposited in Central Greenland As Indicated by Lead Isotopes, Columbia University Academic Commons, .

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